Casillas, now at Porto in the wake of leaving his childhood club a year ago, said things began to harsh with Mourinho amid the 2012-13 season.
That battle was Mourinho's third and last at Real and Casillas said the Portuguese's mentality towards his players changed.
"Our relationship began to change when the group started to slow down in the 2012-2013 season," Casillas told RTVE, through AS.
"Also, you know how these things advance – when everything's going great we can do no wrong – we're all tall, good looking – fundamentally we're the canine's bollocks.
"Be that as it may, when things are going gravely, out of the blue it's what's this? What's all that?
"At last, it's exactly amid those minutes when we you must be more united than any time in recent memory."
Genuine completed the season well afloat of champions Barcelona and Mourinho withdrew, coming back to Chelsea for a brief moment stretch.
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